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Spectroscopic and Electronic Structure Studies of Aromatic Electrophilic Attack and Hydrogen-Atom Abstraction by Non-Heme Iron Enzymes

(4-Hydroxy)mandelate synthase (HmaS) and (4-hydroxyphenyl)pyruvate dioxygenase (HPPD) are two α-keto acid dependent mononuclear non-heme iron enzymes that use the same substrate, (4-hydroxyphenyl)pyruvate, but exhibit two different general reactivities. HmaS performs hydrogen-atom abstraction to... Full description

1st Person: Neidig, Michael L.
Additional Persons: Decker, Andrea verfasserin; Choroba, Oliver W. verfasserin; Huang, Fanglu verfasserin; Kavana, Michael verfasserin; Moran, Graham R. verfasserin; Spencer, Jonathan B. verfasserin; Solomon, Edward I. verfasserin
Source: in Proceedings of the National Academy of Sciences of the United States of America Vol. 103, No. 35 (2006), p. 12966-12973
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Type of Publication: Article
Language: English
Published: 2006
Keywords: research-article
magnetic circular dichroism
density functional calculations
reaction coordinates
Online: Volltext
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